EAP - Proceedings of the Estonian Academy of Sciences

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Technology for the removal of radionuclides from natural water and waste management: state of the art; pp. 122–132

PDF | doi: 10.3176/proc.2013.2.06

Author

Rein Munter

Abstract

The paper provides an overview of natural radionuclides in surface water and groundwater, their maximum permissible concentrations, health effects, different processes of removal (aeration, coagulation and co-precipitation, filtration, adsorption, ion exchange, membrane separation), treatment costs, and options of radioactive waste management.

References

1. Siehl, A. Umweltradioaktivität. Verlag Ernst & Sohn, Berlin, 1996.

2. Wisser, S. Balancing natural radionuclides in drinking water supply. PhD dissertation. Johannes Gutenberg-Universität, Mainz, Germany, 2003.

3. UNSCEAR. Sources and Effects of Ionizing Radiation. United Nations Scientific Committee on the Effects of Atomic Radiation, United Nations Publication, New York, 2000.

4. ICRP. Protection of the Public in Situations of Prolonged Radiation Exposure. ICRP Publication, 82. Pergamon Press, Oxford, New York, 2000.

5. Salonen, L., Turunen, H., Mehtonen, J., Mjönes, L., Hagberg, N., Wilken, R.-D., and Raff, O. Removal of radon by aeration: testing of various aeration techniques for small water works. TENAWA project, EU Contract No. FI4PCT960054, STUK-A193, 2002.

6. Sidhu, K. S. and Breithart, M. S. Naturally occurring ²²⁶Ra and ²²⁸Ra in water supplies of Michigan. Bull. Environ. Contam. Toxicol., 1998, 61, 722–729.
http://dx.doi.org/10.1007/s001289900821

7. Berlin, M. and Rudell, B. Uranium. In Handbook on the Toxicology of Metals (Friberg, L., Nordberg, G. F., and Vouk, V. N., eds). 2nd edn. Elsevier Science Publishers, Amsterdam, 1986, 623–637.

8. Zamora, M. L., Tracy, B. L., Zielinski, J. M., Meyerhof, D. P., and Moss, M. A. Chronic ingestion of uranium in drinking water: a study of kidney bioeffects in humans. Toxicol. Sci., 1998, 43, 68–77.
http://dx.doi.org/10.1093/toxsci/43.1.68

9. World Health Organization. Guidelines for Drinking Water Quality, 3rd edn. Geneva, 2004.

10. Jelinek, R. T. and Sorg, T. J. Operating a small full-scale ion exchange system for uranium removal. J. AWWA, 1988, 80, 79–83.

11. Radioactivity in European Drinking Water. Web-based European Knowledge Network on Water (WEKNOW). 2005.

12. Kiisk, M. Radionukliidide määramise metoodika väljatöötamine Eesti põhjavees [Elaboration of methodology for radionuclides determination in Estonian groundwater]. Report of Project No. 20. Institute of Physics of the University of Tartu, Estonia, 2010.

13. http://www.epa.gov/radiation/tenorm/drinking-water.html (accessed 08.12.2011).

14. http://www.epa.gov/radiation/radionuclides/radon.html#
properties (accessed 08.12.2011).

15. Hess, C. T., Michel, J., and Horton, T. R. The occurrence of radioactivity in public water supplies in the United States. Health Phys., 1985, 48(3), 553–586.
http://dx.doi.org/10.1097/00004032-198505000-00002

16. Raff, O. and Haberer, K. Radon-222 in groundwater in the German Rhine-Nahe area. Vom Wasser, 1998, 90, 311–317.

17. Graves, B. (ed.). Radon in Groundwater. CRC Press, 1987.

18. Crittenden, J. C. (ed.). Water Treatment: Principles and Design. John Wiley, 2005.

19. GDT Manual. Mazzei Corporation, Bakersfield, CA. 2008.

20. Martins, K. L. and Myers, A. G. Controlling radionuclides in water treatment plants: removal, disposal, and exposure minimization. In Proc. of the AWWA Water Quality Technology Conference. New York, 1993, 1077–1109.

21. Annanmäki, M., Turtiainen, T., Jungclas, H., and Rausse, Ch. Disposal of radioactive waste arising from water treatment: recommendations for the EC. Final Report of the WP 8 in the TENAWA project. STUK-A 175, Chapter 8. April, 2000, 61–68.

22. Sorg, T. J. Methods for removing uranium from drinking water. J. AWWA, 1988, 80, 105–111.

23. Havener, M. Radium removal technologies for potable groundwater systems. WaterWorld, 2007, 23(5), 34.

24. Shabana, E. I. and Al-Jaseem, Q. K. Removal of radium from filter sands of a conventional groundwater treatment station. J. Radioanal. Nucl. Ch., 1995, 189(1), 35–43.
http://dx.doi.org/10.1007/BF02040178

25. Vesterbacka, P. and Salonen, L. A case study on removal of natural radionuclides from drinking water using conventional iron and manganese removal equipment. Vatten, 2008, 64(3), 183–191.

26. Moon, D. S., Burnett, W. C., Nour, S., Horwitz, P., and Bond, A. Preconcentration of radium isotopes from natural waters using MnO₂ resin. Appl. Radiat. Isotopes, 2003, 59, 255–262.
http://dx.doi.org/10.1016/S0969-8043(03)00193-3

27. Baeza, A., Salas, A., and Legarda, F. Determining factors in the elimination of uranium and radium from groundwaters during a standard potabilization process. Sci. Total Environ., 2008, 406, 24–34.
http://dx.doi.org/10.1016/j.scitotenv.2008.07.050

28. Lumiste, L., Munter, R., Sutt, J., Kivimäe, T., and Eensalu, T. Removal of radionuclides from Estonian groundwater using aeration, oxidation, and filtration. Proc. Estonian Acad. Sci., 2012, 61, 58–64.
http://dx.doi.org/10.3176/proc.2012.1.08

29. Brinck, W. Radium removal efficiencies in water treatment processes. J. AWWA, 1978, 70, 1–31.

30. http://www.mnawwa.org/about/councils/training/research/radionuclidesremoval.pdf (accessed 08.12.2011).

31. Radium Removal from Potable Water. Tonka Technical Bulletin. Tonka Equipment Company, Plymouth, Minnesota, USA, 2010.

32. www.stuk.fi/julkaisut/stuk-a/stuk-a169.html (accessed 08.12.2011).

33. Valentine, R. L., Splinter, R. C., Mulholland, T. S., Baker, J. M., Nogaj, T. M., and Horng, J. Project Summary: A Study of Possible Economical Ways of Removing Radium from Drinking Water: EPA/600/S2-88/009. US EPA, Washington, April 1988.

34. Pedersen, E. J. Radium removal through co-precipitation with HMO. Water Technology Magazine, 2001, 4(8), 121–136.

35. Clifford, D. and Zhang, Zh. Modifying ion exchange for combined removal of uranium and radium. J. AWWA, 1994, 86, 214–227.

36. Clifford, D., Vijjeswarapu, W., and Subramonian, S. Evaluating various adsorbents and membranes for removing radium from groundwater. J. AWWA, 1988, 80, 94–104.

37. Twinning Light Contract No. EE06-IB-TWP-ESC-03. Estimation of concentrations of radionuclides in Estonian groundwaters and related health risks. Component 1 – Technical Report, April 2009.

38. U.S. Environmental Protection Agency. Office of Drinking Water. Suggested Guidelines for Disposal of Drinking Water Treatment Wastes Containing Naturally Occurring Radionuclides. July, 1990.

39. Cothern, S. A. and Rebers, P. A. Radon, Radium and Uranium in Drinking Water. Lewis Publishers, 1991.

40. Clifford, D. Fundamentals of radium and uranium removal from drinking water. Houston University (www.epa.gov/ogwdw/radionuclides/rads_treatment-dennis-clifford.pdf) (accessed 08.12.2011).

41. U.S. Environmental Protection Agency. National Primary Drinking Water Regulations. Radionuclides: Advanced Notice of Proposed Rulemaking. Fed. Reg. 56, 138–140, CFR Parts 141 and 142, 1991.

42. https://www.riigiteataja.ee/ert.act.jsp?replstring=33&dyn=13223570&id=853253 (accessed 08.12.2011).

43. Hahn, N. A. Disposal of radium removed from drinking water. J. AWWA, 1988, 80, 71–78.

44. IAEA. Application of Ion Exchange Processes for the Treatment of Radioactive Waste and Management of Spent Ion Exchangers. Technical Reports Series No. 408. International Atomic Energy Agency, Vienna, 2002.

45. Kiisk, M., Suursoo, S., Koch, R., Jantsikene, A., and Isakar, K. Radionukliidide määramise metoodika väljatöötamine põhja- ja joogivees [Elaboration of methodology of radionuclides determination in groundwater and drinking water]. Report of Project No. 20. Center of Environmental Investments, 2009 (in Estonian).

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